Basin reactivity:  Determination of solute fate on a basin scale

Temple McKinnon, Department of Geology, University of Montana, Missoula, MT  59812

The Clark Fork River basin in western Montana is an excellent area to study solute metals in contaminated systems. Past flooding events have deposited mine tailings in the river's floodplain. Surface runoff flowing over, and groundwater flowing through, these floodplain deposits provide non-point sources to the dissolved-phase (<0.2 mm), presenting the problem of where to focus remediation resources and efforts.  A basin-wide sampling of the surface water was conducted during the summer of 1998 to determine the transport processes of dissolved-phase metals.  Tributaries of the primary drainages to the basin and with varied mining histories were included in the sampling event.

The headwaters region produced elevated concentrations of As, Cu, Fe, and Mn in surface waters with relatively high pH values (8.5 to 9.2). Treatment ponds downstream from the river's headwaters precipitate trace metals due to the addition of liming agents to the surface water. Most trace element concentrations decrease through this treatment system, with the exception of As.  On a basin-wide scale, the concentration trends for trace elements in the system vary from reactivity to domination by dilution with the surface water discharge of the Clark Fork and its tributaries.  Major ions appear to have downstream sources associated with tributaries or groundwater.  This contrast in concentration trends illustrates the difficulty in studying geochemical trends on the large scale of a basin.

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